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Nakamura, Shoji; Toh, Yosuke; Kimura, Atsushi; Hatsukawa, Yuichi*; Harada, Hideo
Journal of Nuclear Science and Technology, 59(7), p.851 - 865, 2022/07
Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)The present study performed integral experiments of I using a fast-neutron source reactor "YAYOI" of the University of Tokyo to validate evaluated nuclear data libraries. The iodine-129 sample and flux monitors were irradiated by fast neutrons in the Glory hole of the YAYOI reactor. Reaction rates of I were obtained by measurement of decay gamma-rays emitted from I. The validity of the fast-neutron flux spectrum in the Glory hole was confirmed by the ratios of the reaction rates of flux monitors. The experimental reaction rate of I was compared with that calculated with both the fast-neutron flux spectrum and evaluated nuclear data libraries. The present study revealed that the evaluated nuclear data of I cited in JENDL-4.0 should be reduced as much as 18% in neutron energies ranging from 10 keV to 3 MeV, and supported the reported data by Noguere below 100 keV.
Nakano, Masanao
Hoken Butsuri (Internet), 56(1), p.17 - 25, 2021/03
The Tokai Reprocessing Plant is the first reprocessing plant in Japan which started hot test in 1977, and had reprocessed 1140 tons of spent nuclear fuel by May 2007. The gaseous and liquid radioactive wastes has been discharged to the environment. Since iodine-129 (I) is one of the most important nuclides for environmental impact assessment. Therefore, I in the exhaust and effluent has been controlled, and a precise analysis method of I in the environmental samples was developed, and the concentration of 129I in the environment was investigated. This report presents an overview of these activities. Not limited to I on reprocessing facilities, it is essential for nuclear operators to reduce the amount released to the environment in the spirit of ALARA, and to continuously develop the further upgrading environmental monitoring methods and evaluation methods in order to foster a sense of safety and security among residents living in the vicinity of the facilities.
Miwa, Kazuji; Obata, Hajime*; Suzuki, Takashi
Journal of Nuclear Science and Technology, 57(5), p.537 - 545, 2020/05
Times Cited Count:2 Percentile:21.58(Nuclear Science & Technology)This study investigated the vertical distribution of Iodine-129 (I) which is mainly produced by European nuclear reprocessing plants in the Chukchi Sea and Bering Sea. I was found to be distributed almost uniformly in fallout level, and an increasing in I concentration levels caused by high I water inflow from the Atlantic Ocean was not observed. Additionally, we revealed the vertical distribution of iodide, one chemical form of iodine, from the Bering Shelf area to the Chukchi Sea for the first time. The increasing tendency of iodide near sea bottom was observed.
Suzuki, Takashi; Aramaki, Takafumi; Kitamura, Toshikatsu; Togawa, Orihiko
Nuclear Instruments and Methods in Physics Research B, 223-224(1-4), p.87 - 91, 2004/08
Times Cited Count:13 Percentile:63.95(Instruments & Instrumentation)At the Japan Atomic Energy Research Institute, an Accelerator Mass Spectrometer which was installed in Mutsu establishment has two independent beam lines. We verified the precision, the accuracy and the detection limit at this AMS iodine line. Acceptance test for I measurement was carried out on two consecutive days and the I/I ratios obtained during these two days were (7.4970.119) 10 and (7.2090.050) 10 , respectively and the relative standard deviations from the I/I averages per sample were 1.6 % and 0.7 %, respectively. Seawater samples were collected in the western North Pacific and off Rokkasho, Japan before the operation of a nuclear fuel reprocessing plant. Seawater samples preparation for I -AMS measurement was performed by an extraction method. This paper was summarized the performance of this AMS iodine line and measurement results of I/I ratio in seawater samples.
Mineo, Hideaki; Goto, Minoru; Iizuka, Masaru*; Fujisaki, Susumu; Hagiya, Hiromichi*; Uchiyama, Gunzo
Separation Science and Technology, 38(9), p.1981 - 2001, 2003/05
Times Cited Count:22 Percentile:63.74(Chemistry, Multidisciplinary)no abstracts in English
Mineo, Hideaki; Goto, Minoru; Iizuka, Masaru*; Fujisaki, Susumu; Uchiyama, Gunzo
Journal of Nuclear Science and Technology, 39(3), p.241 - 247, 2002/03
Times Cited Count:26 Percentile:82.31(Nuclear Science & Technology)no abstracts in English